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general features. As a consequence, it could be concluded that a significant part of the
variability between models is caused by the description of hydrodynamics. In the case of 137Cs
sediment concentrations, model variability is increased due to the di?erent descriptions of
water–sediment interactions used by each dispersion model.
Exercise 3 consisted of using the same description for water–sediment interactions in the case
of 137Cs. Thus, the same kd, or equivalent kinetic ratios (to be used in cases of equilibrium or
dynamic models respectively), were used. An additional harmonization of models in this
exercise consisted of using exactly the same topographic data for the Pacific Ocean and the
same values for the horizontal and vertical di?usion coe?cients. This experiment was again
carried out for a tracer and for 137Cs. In the latter case, the e?ects of considering the presence
of suspended matter in the water column were also investigated.
In the case of the tracer, agreement between models improved with respect to Exercise 2. The
main factor in producing model discrepancies is water circulation since model agreement
improvement is higher from Exercise 1 to 2 than from Exercise 2 to 3. This confirms a previous
finding where di?erences between models are mainly due to hydrodynamics, although no
systematic study was performed in order to assess this [60].
In the case of 137Cs, the use of the same water–sediment parameterization also led to a better
agreement between model outputs in sediment. Calculated 137Cs concentration maps for water
and sediment were also similar, with models producing the same behaviour. In this respect, it
was also clear that a good description of contamination in the deepest water is essential for a
good description of radionuclide adsorption by bed sediments.
The presence of suspended matter in the water column does not a?ect the calculated dissolved
concentrations. This is not surprising given the relatively low a?nity of 137Cs to be fixed to the
solid phase and the low suspended matter concentration in open ocean waters. E?ectively, for
the considered kd of 137Cs and suspended matter concentration (5 mg/L), the partition coe?cient
indicates that around 99% of this radionuclide remains in solution.
At this stage, given the model harmonization which was carried out, it does not seem possible
to achieve a better agreement between models. Di?erences in model outputs were now due to
intrinsic di?erences between models, i.e.:
? Lagrangian versus Eulerian models;
? Di?erent numerical schemes which may be used for each model category mentioned
above. In this sense, the method used to reconstruct concentrations from the density of
particles in Lagrangian models may be relevant.
Nevertheless, the overall agreement between models which, generally, has been achieved, may
be considered as satisfactory.
The first three exercises assumed a constant hypothetical source of radionuclides. The final
exercise consisted of the use of a realistic source term, allowing the comparison of model
outputs with 137Cs measurements in water and sediment.
The source terms for both direct releases to the Pacific Ocean and atmospheric deposition on
the sea surface had to be reconstructed. The direct release source term was reconstructed by the
JAEA model based on 137Cs measurements carried out by TEPCO at the southern and northern